Issues relating to the complex have been at the center of violence between Israelis and Palestinians in recent weeks.
John Kerry was speaking after talks in Jordan, the formal custodian of what is known to Jews as the Temple Mount and as Haram al-Sharif to Muslims.
He said Israel had renewed a pledge to maintain existing rules there.
In the latest upsurge of violence, at least 8 Israelis have been killed and dozens wounded in knife or gun attacks by Palestinians, following rumors that Israel was planning to change the rules.
About 50 Palestinians, including several of the attackers, have been killed in recent weeks.
John Kerry, who is on a tour of the region, met Palestinian leader Mahmoud Abbas and King Abdullah of Jordan in Amman on October 24.
“All the violence and the incitement to violence must stop. Leaders must lead,” John Kerry told reporters.
The steps he announced include round-the-clock video monitoring and Israel’s agreement to reaffirm Jordan’s historic role as custodian of the religious complex.
Israel says it has not challenged the status quo on the Temple Mount and has no intention of doing so.
John Kerry met Israel’s PM Benjamin Netanyahu on October 22, and said the talks had raised ideas that were worth exploring.
On October 24, John Kerry will travel to Saudi Arabia for talks with regional leaders.
In the latest violence, Israeli police said they shot dead a Palestinian attacker in the northern West Bank on Saturday, October 24.
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